We present sub-ppm sensitivity, broadband gas absorption measurements using improved hollow-core photonic-bandgap
fibers with low loss in the range 3-3.6 μm. The sensitivity levels, unprecedented for a fiber-based sensor system, were
achieved by addressing the strong mid-IR vibrational bands through use of a high-intensity supercontinuum source and
by exploiting long interaction lengths in the HC-PBGFs. We measured mixtures of methane (1034 ppm) and ethane
(50.4 ppm) and attained 7 and 0.9 ppm sensitivities for 0.925 and 5.69 m long HC-PBGF samples, respectively, from
high-resolution (0.2 nm) spectra. Significant scope for further sensitivity improvement exists through use of longer fibers
in combination with more sophisticated sensing schemes.
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