Optically nonlinear effects in bulk chiral nematic NLO-polymers: second harmonic generation in chiral nematic polymer films

Gustaaf R. Moehlmann; H. W. Berendse; M. Bosma; Koen J. Clays; Thierry Verbiest; Martti Kauranen; Jeffery J. Maki; Andre P. Persoons

doi:10.1117/12.222807

5 October 1995 Optically nonlinear effects in bulk chiral nematic NLO-polymers: second harmonic generation in chiral nematic polymer films

Gustaaf R. Moehlmann, H. W. Berendse, M. Bosma, Koen J. Clays, Thierry Verbiest, Martti Kauranen, Jeffery J. Maki, Andre P. Persoons

Author Affiliations +

Proceedings Volume 2527, Nonlinear Optical Properties of Organic Materials VIII; (1995) https://doi.org/10.1117/12.222807
Event: SPIE's 1995 International Symposium on Optical Science, Engineering, and Instrumentation, 1995, San Diego, CA, United States

Abstract

We report on a novel class of optically nonlinear polymeric materials realized by processing onto a substrate a combination of molecules and polymers comprising hyperpolarizable and thus optically nonlinear molecular groups, liquid crystal moieties, and chiral moieties. Since processing of this combination of materials leads to a spontaneously noncentrosymmetric bulk orientation of the hyperpolarizable moieties in its thermodynamically most stable state, the material exhibits second-order nonlinear-optical properties that can be used for second-order nonlinear-optical effects such as frequency doubling of optical radiation, the linear electro- optic of Pockels effects, magneto-optic effect, nonlinear dichroism, etc. We will present and discuss the experimental results concerning the nonlinear-optical properties obtained via frequency doubling of light in these materials.

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Gustaaf R. Moehlmann, H. W. Berendse, M. Bosma, Koen J. Clays, Thierry Verbiest, Martti Kauranen, Jeffery J. Maki, and Andre P. Persoons "Optically nonlinear effects in bulk chiral nematic NLO-polymers: second harmonic generation in chiral nematic polymer films", Proc. SPIE 2527, Nonlinear Optical Properties of Organic Materials VIII, (5 October 1995); https://doi.org/10.1117/12.222807

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