Ultrafast Raman echo experiments in the liquid phase

Mark A. Berg; Laura J. Muller; David A. Vanden Bout

doi:10.1117/12.58168

1 April 1992 Ultrafast Raman echo experiments in the liquid phase

Mark A. Berg, Laura J. Muller, David A. Vanden Bout

Proceedings Volume 1638, Optical Methods for Time- and State-Resolved Chemistry; (1992) https://doi.org/10.1117/12.58168
Event: OE/LASE '92, 1992, Los Angeles, CA, United States

Abstract

The Raman echo experiment, which can distinguish homogeneous and inhomogeneous broadening of vibrational spectra, is reported for the first time in liquids. The symmetric methyl stretch of acetonitrile, which has been extensively studied with contradictory results, is shown to be homogeneously broadened. The vibration interacts only with rapid collisional motions of the solvent.

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Mark A. Berg, Laura J. Muller, and David A. Vanden Bout "Ultrafast Raman echo experiments in the liquid phase", Proc. SPIE 1638, Optical Methods for Time- and State-Resolved Chemistry, (1 April 1992); https://doi.org/10.1117/12.58168

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