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Nonlinear interferometers based on correlated photon pairs allow mid-infrared spectroscopy by measuring only near-infrared photons with a silicon-based detector, which offers higher detectivities than mid-infrared detectors. Here, we use the nonlinear interferometer not only to determine the transmission of a sample but also for spectral analysis – analogue to classical Fourier transform infrared (FTIR) spectrometers. The Quantum FTIR analyzes the absorption of gas mixtures with high spectral resolution over a broad mid-infrared wavelength range. Improved emission rates of the photon pair source yield sensitivities similar to a classical FTIR despite an extremely low light exposure on the sample.
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Jachin Kunz, Chiara Lindner, Simon J. Herr, Sebastian Wolf, Jens Kiessling, Frank Kühnemann, "High resolution Fourier-transform mid-infrared spectroscopy using nonlinear interferometers," Proc. SPIE 12447, Quantum Sensing, Imaging, and Precision Metrology, 124471A (8 March 2023); https://doi.org/10.1117/12.2650157