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Different frequency conversion processes in the mid-IR were experimentally studied with slab RF discharge CO and CO2 lasers and various nonlinear crystals ZnGeP2, GaSe, BaGa2GeSe6, AgGaSe2 and PbIn6Te10 : second and third harmonic generation of CO laser; sum and difference frequency generation of CO and CO2 lasers. Mid-IR emission on hundreds of narrow spectral lines from 1.7 μm to 19.3 μm was obtained
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Andrey Ionin, Igor Kinyaevskiy, Yurii Klimachev, Andrei Kotkov, Andrei Kozlov, Adilya Sagitova, Leonid Seleznev, Dmitry Sinitsyn, "Hybrid molecular gas laser systems operating within wavelength range of 1.7–19.3 micron," Proc. SPIE 11162, High Power Lasers: Technology and Systems, Platforms, Effects III, 111620D (7 October 2019); https://doi.org/10.1117/12.2532492